Photon-in photon-out hard X-ray spectroscopy at the Linac Coherent Light Source

Alonso-Mori, R.; Sokaras, D.; Zhu, D.; Kroll, T.; Chollet, M.; Feng, Y.; Glownia, J.M.; Kern, J.; Lemke, H.T.; Nordlund, D.; Robert, A.; Sikorski, M.; Song, S.; Weng, T.-C.; Bergmann, U.

doi:10.1107/S1600577515004488

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Figure 5
Time-dependent photo-induced Fe $[K\beta]$ difference spectra (b) and kinetic modelling of spin crossover dynamics [(a) and (c)] for Fe(bpy)₃. After excitation into the metal–ligand charge transfer state, transition into the HS ⁵T₂ state [inset in (c)] causes an increase of the Fe-to-ligand distance [inset in (a)]. The difference signal measured at a $[K\beta]$ fluorescence energy of 7061 eV [(a) green diamonds] and 7054 eV [(c) black symbols]. The data have been overlaid with results from global fits including (blue lines) and excluding (green dashed lines) population of and intermediate ³T₂ triplet state. Courtesy of Zhang et al. (2014)

JOURNAL OF
SYNCHROTRON
RADIATION

ISSN: 1600-5775

Volume 22| Part 3| May 2015| Pages 612-620

https://doi.org/10.1107/S1600577515004488

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