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ISSN: 1600-5775

Analytic expressions for the angular and the spectral fluxes at Compton X-ray sources

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aLaboratoire de l'Accélérateur Linéaire, Orsay, France
*Correspondence e-mail: [email protected]

Edited by M. Yamamoto, RIKEN SPring-8 Center, Japan (Received 21 April 2016; accepted 26 October 2016)

The goal of this paper is to express simply the number of photons impinging on a target in the framework of accelerator-based Compton X-ray sources. From the basic kinematics of Compton sources, analytic formulas for the angular and the spectral fluxes are established as functions of the energy spread or/and the angular divergence of the electron and the laser beams. Their detailed predictions are compared with Monte Carlo simulations. These analytic expressions allow one to compute in a simple and precise way the X-ray flux in a given angular acceptance and a given energy bandwidth, knowing the characteristics of the incoming beams.

1. Introduction

Today, Compton X-ray sources are in full development thanks to the exceptional improvement of high-power lasers over the last 15 years. The principle is based on the production of X-ray pulses of a few tens of keV in energy by Compton backscattering of intense laser light of micrometric wavelength against an electron bunch of tens of MeV in energy (i.e. about 100 times less energetic than electrons used to produce synchrotron radiation in the X-ray range). Such Compton sources are compact installations (with areas of ∼100 m2) which provide high-intensity, high-quality X-ray beams with a tunable energy. The present most ambitious projects aim at producing a total flux of 1012 1014 photons s−1 (Jacquet, 2014[Jacquet, M. (2014). Nucl. Instrum. Methods Phys. Res. B, 331, 1-5.]) that gives access to experimental methods currently used at synchrotron beamlines. For various applications, the development of these sources will allow the use of powerful analysis techniques in such environments as hospitals, laboratories or museums. The diversity of the possible applications of these sources increases the demand for a simple formulation of the X-ray flux available at a target sample with an intuitive understanding of its spectral and spatial properties. Our motivation is to guide the users when evaluating the performances of such sources in their domain of competence (medical, materials, art history, etc.). Indeed, to our knowledge, there is no analytic formulas in the literature describing angular and spectral X-ray fluxes expected from a given Compton source. There are some analogies between synchrotron radiation sources and Compton sources, but the spectral and the spatial properties are different. Thus, Compton backscattering sources need a specific description. Our analytic formulas provide the flux within a finite polar angle around the electron beam direction and within a finite bandwidth around the Compton edge. The energy spread and the angular divergence of the electron beam and of the laser affect the X-ray flux in the chosen kinematic region. The estimation of such effects is the purpose of this article. The analytic expressions are obtained by convolving purely kinematic effects with expressions that characterize the laser and the electron beam properties.

The basic principles of a Compton source, the kinematics and our calculation framework are described in §2[link]. The performances of current laser systems are such that the main impact on the Compton source characteristics comes from the angular divergence Mathematical equation and the energy spread Mathematical equation of the incident electron beam. The latter may vary widely depending on the chosen accelerator complex (see §2.2[link]). Analytic expressions for the total X-ray flux and for its angular and spectral dependences are established in §3[link] and §4[link] as functions of these two electron beam parameters and compared with Monte Carlo simulations.

2. Key parameters for the X-ray flux

This section introduces the key parameters needed to understand the analytic developments that follow.

2.1. The Compton process

Fig. 1[link] describes the Compton scattering between a free relativistic electron of Lorentz factor γ and a photon of energy Mathematical equation which is the basic process exploited in an accelerator-based X-ray source.

[Figure 1]
Figure 1
Schematic drawing of the scattering process between an electron and a laser photon. xyz is the laboratory frame.

Electrons of a few tens of MeV are used in X-ray sources whereas the laser is usually in the infrared domain. In the laboratory frame, the scattered photon energy Mathematical equation varies quadratically with the electron energy and linearly with the laser photon energy Mathematical equation. Assuming Mathematical equation and the laser photon energy is small compared with the electron rest mass energy, we can derive from the kinematics of the process

Mathematical equation

where Mathematical equation is the collision angle and Mathematical equation the scattering polar angle of the Compton photon with respect to the incoming electron momentum. Equation (1a)[link] implies an univocal dependence between the energy of the backscattered photon and its emission angle Mathematical equation. Photons of maximum energy Mathematical equation are those emitted on-axis (Mathematical equation = 0°). For an X-ray which is produced by an electron of Lorentz factor γ, let ɛ be the ratio of Mathematical equation and Mathematical equation. The dependence on ɛ of the normalized differential cross section Mathematical equation can be expressed as (Telnov, 2000[Telnov, V. (2000). Nucl. Instrum. Methods Phys. Res. A, 455, 80-89.])

Mathematical equation

Equations (1a), (1b)[link], (2a) and (2b)[link] will be the key relations used to establish the analytic expressions for the X-ray flux in a given spectral bandwidth or/and within a given angular acceptance, and to quantify the reduction of the angular and spectral fluxes due to the energy spread and the angular divergence of the two colliding beams.

The Compton X-ray sources involve multi-collisions between a laser pulse and an electron bunch. Thus, to establish the total X-ray flux, we need to take into account the laser pulse and the electron bunch sizes. Let Mathematical equation and Mathematical equation be, respectively, the number of electrons per bunch and the number of photons per laser pulse, and let Mathematical equation, Mathematical equation and Mathematical equation be the transverse and longitudinal dimensions (r.m.s.) of the electron bunch and laser pulse at the interaction point. Assuming the electron beam and the laser have Gaussian distributions in the three dimensions, for electron–photon collisions taking place with a crossing angle Mathematical equation in the xz plane, the number of X-ray produced per second is (Suzuki, 1976[Suzuki, T. (1976). KEK Technical Report 76-3, July 1976. KEK, Tsukuba, Japan.])

Mathematical equation

Mathematical equation is proportional to the Thomson cross section Mathematical equation, the luminosity and the repetition frequency of the interactions Mathematical equation. High X-ray fluxes are foreseen in various projects. For example, ThomX (Variola et al., 2014[Variola, A., Haissinkski, J., Loulergue, A. & Zomer, F. (2014). ThomX Technical Design Report. LAL/RT 14-21. SOLEIL/SOU-RA-3629.])) foresees F(0) ≃ 1013 photons s−1 with Mathematical equation = 45 keV for a 50 MeV electron bunch (Mathematical equation = 100) of 1 nC, micrometric wavelength laser pulses of 10 mJ, Mathematical equation = 20 MHz, and Mathematical equation ≃ 40 µm.

Expression (3)[link] will be our reference flux hereafter referred to as Mathematical equation.

2.2. X-ray spectral bandwidth

Relations (1a) and (1b)[link] imply that the X-ray energy spectrum produced by electrons and photons whose energies are single-valued is strictly monochromatic at a given emission angle. But the energy dispersion and the angular divergence of the stored electrons and, to a lesser extent, of the photons at the interaction point lead to a significant broadening of Mathematical equation at a given scattering angle Mathematical equation.

The relative energy spreads (r.m.s.) of an electron bunch and of a laser pulse will be denoted by Mathematical equation and Mathematical equation, while their angular divergences (r.m.s.) will be denoted by Mathematical equation and Mathematical equation (assuming that the horizontal and the vertical divergences are equal). The order of magnitude of the broadening Mathematical equation of the on-axis Compton spectrum due to each one of these four parameters can be estimated from equations (1a) and (1b)[link] by replacing γ, Mathematical equation, Mathematical equation and Mathematical equation with Mathematical equation, Mathematical equation, Mathematical equation and Mathematical equation, respectively, and performing four Taylor series expansions of equation (1a)[link] in Mathematical equation, Mathematical equation, Mathematical equation and Mathematical equation, resulting in: Mathematical equation Mathematical equation Mathematical equation, Mathematical equation Mathematical equation Mathematical equation, Mathematical equation Mathematical equation Mathematical equation and Mathematical equation Mathematical equation Mathematical equation due to Mathematical equation, Mathematical equation, Mathematical equation and Mathematical equation, respectively.

We will give now orders of magnitude for these Mathematical equation, Mathematical equation, Mathematical equation and Mathematical equation parameters for current electron guns and pulsed lasers:

(i) The normalized horizontal and vertical emittances Mathematical equation and Mathematical equation of ∼1 nC bunches delivered by good quality current electron guns are 1–5 mm mrad (Arnold & Teichert, 2011[Arnold, A. & Teichert, J. (2011). Phys. Rev. ST Accel. Beams 14, 024801.]; Rao & Dowell, 2013[Rao, T. & Dowell, D. H. (2013). An Engineering Guide to Photoinjectors, https://arxiv.org/ftp/arxiv/papers/1403/1403.7539.pdf.]). With these values, transverse sizes and normalized divergences are typically Mathematical equation ≃ 20–100 µm and Mathematical equation ≃ 0.01–0.25 rad, respectively.

(ii) Concerning Mathematical equation, the electron beam relative energy spread, current values at electron accelerators are of a few Mathematical equation up to a few percent.

(iii) On the laser side, the product of Mathematical equation, the r.m.s. energy bandwidth of the pulse, and Mathematical equation, its r.m.s. temporal duration, is constrained by the uncertainty principle (Donnelly & Grossman, 1998[Donnelly, T. D. & Grossman, C. (1998). Am. J. Phys. 66, 677.]) Mathematical equation Mathematical equation Mathematical equation. Unchirped pulses have the minimum time-bandwidth product, i.e. close to Mathematical equation, whereas larger values prevail for chirped pulses. Then, let us consider a laser with a wavelength λ, and an r.m.s. pulse duration Mathematical equation. Assuming unchirped pulses, one derives from the uncertainty principle: Mathematical equation Mathematical equation Mathematical equation = Mathematical equation, where c is the speed of light. It follows that infrared fs–ps pulses have a relative energy spread Mathematical equation of a few Mathematical equation (for 10 ps pulses) up to a few Mathematical equation (for 100 fs pulses).

(iv) In good quality lasers with Gaussian pulses, the relation between the r.m.s. transverse pulse sizes Mathematical equation, Mathematical equation and the angular divergence Mathematical equation is Mathematical equation = Mathematical equation = Mathematical equation (Schmüser et al., 2008[Schmüser, P., Dohlus, M. & Rossbach, J. (2008). Ultraviolet and Soft X-ray Free-Electron Lasers. Berlin: Springer.]), leading to the following typical values: Mathematical equation ≃ 10–100 µm and Mathematical equation ≃ 1–10 mrad (infrared laser).

Table 1[link] summarizes these orders of magnitude and the corresponding broadening of the Compton spectrum Mathematical equation. The spectrum broadening due to the laser bandwidth Mathematical equation is negligible, as well as the broadening due to the laser divergence if the product Mathematical equation is smaller than ∼1 mrad, which is the case in almost all current Compton projects where electrons and laser photons collide head-on (Jacquet, 2014[Jacquet, M. (2014). Nucl. Instrum. Methods Phys. Res. B, 331, 1-5.]). We conclude that Mathematical equation is mainly governed by the angular divergence and the relative energy spread of the electron beam.

Table 1
Orders of magnitude of the relative energy spread and divergence of electron and laser beams at the interaction point, and associated broadening of the Compton spectrum

Variable Typical values Mathematical equation
Mathematical equation Mathematical equationMathematical equation Mathematical equationMathematical equation
Mathematical equation Mathematical equationMathematical equation Mathematical equationMathematical equation
Mathematical equation 0.01–0.25 Mathematical equationMathematical equation
Mathematical equation 1–10 Mathematical equationMathematical equation (Mathematical equation
Mathematical equationMathematical equation (Mathematical equation ≃ 1–10 mrad)

2.3. Input and notations

In this section, we introduce the probability distributions used to establish the analytic expressions of §3[link] and §4[link]. The nominal Lorentz factor of the electron beam will be referred to as Mathematical equation. Then the Lorentz factor of a given electron is written as Mathematical equation = Mathematical equation, where Mathematical equation is the difference in energy of this electron with respect to the nominal beam energy ( E0) divided by E0. With Mathematical equation being the nominal value of the crossing angle between the electron beam and the laser in the xz plane (see Fig. 1[link]), we define Mathematical equation, Mathematical equation, Mathematical equation and Mathematical equation as the angles to z axis of the projections of the momentum of a given electron and of a given laser photon in the xz and yz planes. The probability distributions of Mathematical equation, Mathematical equation and Mathematical equation are assumed to be Gaussian with standard deviations Mathematical equation, Mathematical equation and Mathematical equation, respectively. We further assume Mathematical equation = Mathematical equation = Mathematical equation and Mathematical equation = Mathematical equation = Mathematical equation. Mathematical equation (Mathematical equation, respectively) is defined as the convolution of the Mathematical equation and Mathematical equation distributions (of Mathematical equation and Mathematical equation, respectively) and follows a Gaussian distribution whose standard deviation is Mathematical equation = Mathematical equation.

We introduce also the polar and azimuthal angles with respect to the z-axis direction (see Fig. 2[link]), Mathematical equation and Mathematical equation, of an electron momentum (Mathematical equation = Mathematical equation, Mathematical equation = Mathematical equation, Mathematical equation = Mathematical equation), and similarly Mathematical equation and Mathematical equation for a photon scattered by this electron. For small Mathematical equation and Mathematical equation (i.e. when Mathematical equationMathematical equation and Mathematical equationMathematical equation), the polar angle Mathematical equation of the backscattered photon with respect to the electron momentum is Mathematical equation = Mathematical equation + Mathematical equation Mathematical equation Mathematical equation. Summing over azimuthal angles we obtain

Mathematical equation

The Mathematical equation angle averaged over Mathematical equation and Mathematical equation expressed in (4)[link] is the one that appears in equation (1a)[link].

[Figure 2]
Figure 2
Polar angles of an electron momentum (Mathematical equation) and of a Compton photon (Mathematical equation) scattered by this electron with respect to the z-axis, and polar angle Mathematical equation of the Compton photon with respect to the electron momentum. Note that the electron momentum is practically not affected by the collision.

Explicitly, the probability distributions of Mathematical equation, Mathematical equation and Mathematical equation defined in the ranges Mathematical equation, Mathematical equation and Mathematical equation, respectively, are

Mathematical equation

In the following sections we will obtain analytic expressions for the ratios Mathematical equation = Mathematical equation, Mathematical equation = Mathematical equation, Mathematical equation = Mathematical equation and Mathematical equation = Mathematical equation, where Mathematical equation is the total flux, Mathematical equation the flux in a given angular acceptance α (of a few milliradians) around the z-axis direction, Mathematical equation the flux in a given energy bandwidth (bw) centered at the on-axis X-ray energy Mathematical equation = Mathematical equation, and Mathematical equation the flux in a given angular acceptance and a given energy bandwidth. We will study the dependence of these ratios on the Mathematical equation and Mathematical equation parameters which govern the broadening of the Compton angular spectrum as discussed in §2.2[link], and we will confront our formulas with simulations performed with the CAIN code (Yokoya, 2003[Yokoya, K. (2003). User's Manual of CAIN, https://lcdev.kek.jp/~yokoya/CAIN/cain235/CainMan235.pdf. ]) generated with several Mathematical equation and Mathematical equation values, all other parameters (Mathematical equation, Mathematical equation, Mathematical equation Mathematical equation, Mathematical equation, Mathematical equation, Mathematical equation, Mathematical equation and Mathematical equation) remaining fixed. In the CAIN simulations, we use Mathematical equation = 100 (i.e. the order of magnitude to produce Compton backscattered photons in the X-ray domain), a laser wavelength Mathematical equation = 1 µm, and we assume a pulse waist of 40 µm. For a full range coverage of the electron beam parameters in current accelerators (see Table 1[link]), the Mathematical equation and Mathematical equation ranges used for this work are Mathematical equation ≃ 0.01–0.25 rad (i.e. Mathematical equation ≃ 0–2.5 mrad for Mathematical equation ≃ 100) and Mathematical equation ≃ 0–2%.

3. Spectral or angular selection

In this section, we will obtain the expression of the X-ray flux when one selects either the energy or the emission angle of the X-rays.

3.1. Dependence of the total flux Ftot on the electron and the laser beam angular divergences

Since we assume here that no cut is applied to the X-ray energy, the electron beam energy spread does not come into this calculation. Thus we treat here only the electron beam and the laser beam divergences. We consider the collision of an electron with a photon at a nominal crossing angle Mathematical equation in the horizontal plane xz. The effect of the two Mathematical equation and Mathematical equation variables (defined in §2.3[link]) can be treated as an additional contribution to Mathematical equation. Indeed, for small Mathematical equation and Mathematical equation (i.e. when Mathematical equationMathematical equation and Mathematical equationMathematical equation) and by making the approximation that Mathematical equation and Mathematical equation are awarded only to the electron (see Fig. 3[link]), a geometrical calculation leads to an effective electron–photon crossing angle Mathematical equation such that Mathematical equation = Mathematical equation + Mathematical equation

[Figure 3]
Figure 3
Nominal (Mathematical equation) and effective (Mathematical equation) electron–photon crossing angles assuming that Mathematical equation and Mathematical equation are awarded only to the electron.

Then, for an electron bunch and a laser pulse of r.m.s. angular divergence Mathematical equation and Mathematical equation, respectively, the total flux Mathematical equation Mathematical equation Mathematical equation is obtained by integrating Mathematical equation, weighted by the Gaussian probabilities of Mathematical equation and Mathematical equation [see equation (5b)[link]]. Keeping up to the second-order terms in Mathematical equation and Mathematical equation results in the following expression for the ratio Mathematical equation Mathematical equation Mathematical equation:

Mathematical equation

where rxz = Mathematical equation. For Mathematical equation = 72 µm, Mathematical equation = 40 µm, Mathematical equation = 4.8 mm, Mathematical equation = 3 mm and Mathematical equation = 2 mrad (i.e. the laser beam divergence value corresponding to a 40 µm waist size), Mathematical equation is shown in Fig. 4[link] as a function of Mathematical equation, for Mathematical equation = 0°, 1° and 2°, and compared with results obtained with the CAIN simulation program. The analytic expression reproduces well the differences between the various collision angle cases. A reduced collision angle amplifies the divergence impact on the total flux but only to a small extent, less than 1% for head-on collisions.

[Figure 4]
Figure 4
The ratio Mathematical equation = Mathematical equation as a function of Mathematical equation for a laser divergence Mathematical equation = 2 mrad, for Mathematical equation = 0° (black bullets, black line), 1° (red squares, red line) and 2° (blue open circle, blue line). Points are CAIN simulations. For each point, the error bar indicates the statistical uncertainty calculated from the number of generated events (namely ∼4.7 × 105, 4.1 × 105 and 3.1 × 105 events for each of the eight points generated with Mathematical equation = 0°, 1° and 2°, respectively). Lines illustrate the analytic formula [equation (6)[link]] results.

3.2. X-ray flux in a given energy bandwidth (Fbw)

In this section we look at the number of X-rays produced when an energy cut is applied. For this, the electron energy spread is decisive whereas Mathematical equation is independent of the electron beam angular divergence since no angular selection is assumed here. Also, we do not take into account the broadening of the Compton spectrum (Mathematical equationMathematical equationMathematical equation) that occurs in the particular case where both the laser divergence and the collision angle are large (see Table 1[link]).

Let us consider an electron of Lorentz factor Mathematical equation = Mathematical equation. The energy of a photon which is backscattered by this electron is Mathematical equation and, according to equation (1b)[link], the maximum value of Mathematical equation is Mathematical equation = Mathematical equation where Mathematical equation = Mathematical equation. The ratio Mathematical equation is denoted by Mathematical equation. Mathematical equation is the flux of photons whose Mathematical equation lies in the interval between 1 − bw and 1 + bw. The energy probability distribution (2a)[link] expressed as a function of Mathematical equation becomes

Mathematical equation

Fig. 5[link] shows this distribution for three different cases: Mathematical equation < 0, Mathematical equation = 0 and Mathematical equation > 0. Since Mathematical equation is a quasi-linear function for Mathematical equation larger than ∼0.65, the integral of Mathematical equation between Mathematical equation and Mathematical equation can be approximated by Mathematical equation. Thus Mathematical equation is calculated in the following way (see Fig. 5[link]):

[Figure 5]
Figure 5
Differential cross section Mathematical equation for three electron populations: electrons with positive Mathematical equation (dotted line), with Mathematical equation = 0 (solid line), and with negative Mathematical equation (dashed line), as a function of the scattered photon energy Mathematical equation = Mathematical equation. Also represented are Mathematical equation (green area) and Mathematical equation (area hatched in green).

(i) Electrons with Mathematical equation such that Mathematical equation < 1 − bw do not contribute to Mathematical equation.

(ii) The contribution to Mathematical equation of electrons having a relative energy difference Mathematical equation such that 1 − bw < Mathematical equation < 1 + bw is denoted by Mathematical equation and is equal to the integral of Mathematical equation between Mathematical equation = 1 − bw and Mathematical equation = Mathematical equation (green area): Mathematical equation = Mathematical equation. These electrons are denoted by Mathematical equation in Fig. 5[link].

(iii) The contribution of electrons whose Mathematical equation satisfies 1 + bw < Mathematical equation is denoted by Mathematical equation and is equal to the integral of Mathematical equation between Mathematical equation = 1 − bw and Mathematical equation = 1 + bw (area hatched in green): Mathematical equation = Mathematical equation. These electrons are denoted by Mathematical equation in Fig. 5[link].

Assuming that the Mathematical equation variable follows the Gaussian distribution (5a)[link] where Mathematical equation ≃ 0–2%, one can make the approximation Mathematical equationMathematical equation and Mathematical equation can be written

Mathematical equation

Performing a first-order Taylor expansion in Mathematical equation, the calculation of the above integrals leads to

Mathematical equation

and is shown in Fig. 6[link] as a function of Mathematical equation, for three energy bandwidths: (a) bw = 0.1%, (b) bw = 0.7% and (c) bw = 3%.

[Figure 6]
Figure 6
The ratio Mathematical equation = Mathematical equation as a function of Mathematical equation for three energy bandwidths: (a) bw = 0.1%, (b) bw = 0.7% and (c) bw = 3%. Points are CAIN simulations and the error bars indicate the statistical uncertainties. Lines are obtained using the analytic formula (8)[link].

First of all, in the absence of any energy spread, one notes a factor 3/2 compared with the classical formula used for synchrotron radiation, showing the need for a proper analytic development when dealing with Compton sources. This factor, which comes from the Compton cross section, remains whatever the selected energy acceptance. Fig. 6[link] shows that a linear behavior of the flux reduction with Mathematical equation prevails if the selected bandwidth is small compared with Mathematical equation (as in the 0.1% and 0.7% cases and in the right-hand region of the 3% case), whereas the flux remains globally constant when the energy acceptance is large with respect to Mathematical equation (as in the left-hand region of the 3% case). In the three bandwidth cases, the small systematic difference between the CAIN simulation values and the analytic results for Mathematical equation ≃ 2% shows that higher-order terms in Mathematical equation have to be taken into account for Mathematical equation values larger than 2–3%. In any event, the reduction due to the energy spread is less than 10% in the parameter range considered here.1

3.3. X-ray flux in a given angular acceptance

We now consider the photon flux Mathematical equation within a given angular acceptance α. In this case, the effect of an energy spread is completely negligible since the mean value of Mathematical equation vanishes.

For any value of the polar angle θ, the Mathematical equation product is denoted as Mathematical equation. Let us consider an electron whose momentum makes a polar angle Mathematical equation with respect to the z axis (see Fig. 2[link]) while the photon backscattered by this electron has a polar angle Mathematical equation. Using equations (1a)[link], (2a)[link] and (4)[link], the dependence of the normalized differential Compton cross section on Mathematical equation is given by

Mathematical equation

This distribution is shown in Fig. 7[link] for Mathematical equation = 0 and Mathematical equation = 0.04. Here again, with Mathematical equation being a quasi-linear function of Mathematical equation for Mathematical equation smaller than ∼0.15, its integral between Mathematical equation and Mathematical equation can be approximated by Mathematical equation. Then, as illustrated by Fig. 7[link], an electron contribution to Mathematical equation is equal to Mathematical equation and, according to the exponential distribution (5c)[link] of Mathematical equation, the ratio Mathematical equation for an electron bunch of r.m.s. divergence Mathematical equation = Mathematical equation = Mathematical equation can be simply expressed as

Mathematical equation

The calculation of equation (10)[link] using a first-order Taylor series expansion in Mathematical equation leads to

Mathematical equation

Expression (11)[link] is valid as long as Mathematical equation and Mathematical equation are less than ∼0.15 and ∼0.03, respectively. For larger values of Mathematical equation, the linear approximation of Mathematical equation is no longer valid and the integral between 0 and Mathematical equation must be explicitly calculated. For Mathematical equation Mathematical equation 0.03, higher-order terms in Mathematical equation have to be taken into account in the series expansion of equation (10)[link]. Mathematical equation and points obtained with CAIN are shown in Fig. 8[link] as a function of Mathematical equation (for Mathematical equation = 100) for an anglular acceptance α of 1 mrad and 2 mrad. Equation (11)[link] is represented by the solid lines and is in very good agreement with CAIN simulations up to Mathematical equation ≃ 1.5 mrad. The need to take into account higher-order terms in Mathematical equation in the modeling of Mathematical equation for large values of Mathematical equation is highlighted for Mathematical equation ≃ 2 mrad. The dotted lines indicate the analytic expression results when the third-order term in Mathematical equation is taken into account.2

[Figure 7]
Figure 7
The angular differential cross section Mathematical equation as a function of Mathematical equation for Mathematical equation = 0 (solid line) and for Mathematical equation = 0.04 (dashed line). The shaded area shows the contribution to Mathematical equation of an electron whose momentum has a polar angle Mathematical equation.
[Figure 8]
Figure 8
The ratio Mathematical equation = Mathematical equation as a function of Mathematical equation for an angular acceptance Mathematical equation of 1 mrad (open red circles and red line) and 2 mrad (black bullets and black line). Points are CAIN simulations (the error bars are too small to be visible). Solid lines are obtained with equation (11)[link], dotted lines show Mathematical equation calculated to third order in Mathematical equation.

4. X-ray flux within a given angular acceptance and a given energy bandwidth

In this section we assume that both an angular cut and an energy selection are applied to the backscattered photons and we calculate the consequent reduction of the X-ray flux. In the first two subsections, the electron beam divergence and its energy spread will be treated independently to understand the impact of each one of these parameters. Then we will take into account both of these beam characteristics.

4.1. Dependence on the electron beam angular spread

Our starting point is equation (8)[link] which gives the X-ray yield in a given energy bandwidth, and we will modify this expression to take into account the angular acceptance defined by a maximum value α of the X-ray emission direction with respect to the z axis and the electron beam angular spread. In order to achieve a single formulation, we associate an angle to the energy bandwidth, namely Mathematical equation = Mathematical equation. At this stage, we have to treat separately the Mathematical equation < Mathematical equation case and the Mathematical equation > Mathematical equation case, as illustrated in Fig. 9[link]. The dashed red line represents the electron momentum direction which makes an angle Mathematical equation with respect to the z direction. α defines the angular cut and Mathematical equation the energy acceptance translated into an angle. More precisely, to the energy bandwidth (or energy acceptance) bw corresponds an angular acceptance which is a cone whose axis is the momentum of the electron which backscatters the incoming photon and whose half aperture is Mathematical equation. In Fig. 9[link], those X-rays which pass both the angular and the energy cuts are the ones emitted in the green domain. The hatched regions show emission directions which are outside the X-ray angular acceptance cone of aperture α. The accepted region depends on the three angles involved in the following way:

[Figure 9]
Figure 9
Top: the Mathematical equation > Mathematical equation case where Mathematical equation = Mathematical equation. Three configurations are shown: (a) Mathematical equation < Mathematical equation, (b) Mathematical equation < Mathematical equation < Mathematical equation, (c) Mathematical equation < Mathematical equation < Mathematical equation. Bottom: the Mathematical equation < Mathematical equation case. (d) Mathematical equation < Mathematical equation, (e) Mathematical equation < Mathematical equation < Mathematical equation, (f) Mathematical equation < Mathematical equation < Mathematical equation.

(i) For Mathematical equation > Mathematical equation (see upper panels in Fig. 9[link]) and values of Mathematical equation such that Mathematical equation < Mathematical equation, all the X-rays whose energy belong to the accepted bandwidth pass the angular cut [case (a)]; when Mathematical equation increases, the cone intersection diminishes and depends on whether Mathematical equation is larger than α or not [(b) and (c) cases];

(ii) For Mathematical equation < Mathematical equation (see lower panels in Fig. 9[link]), the cone intersection is reduced as the electron angular spread increases and depends on whether Mathematical equation is larger than Mathematical equation or not [(e) and (f) cases].

To take into account the various cases enumerated above, we introduce the following two angles: Mathematical equation = Mathematical equation and Mathematical equation = Mathematical equation. Then, using the Mathematical equation probability distribution of equation (5c)[link], an integration is performed for each of the three cases and the number of X-rays backscattered in the angular acceptance α and within a given energy bandwidth bw is given by the following expression:

Mathematical equation

where Mathematical equation is given by equation (8)[link] with Mathematical equation ≃ 0, i.e. Mathematical equation = Mathematical equation. Equation (12)[link] leads to the following analytic expression for Mathematical equation:

Mathematical equation

CAIN simulations and results from equation (13)[link] are shown in Fig. 10[link] where Mathematical equation is plotted against the angular divergence Mathematical equation for several values of the acceptance angle α and several values of the energy bandwidth bw.

[Figure 10]
Figure 10
The ratio Mathematical equation = Mathematical equation plotted as a function of Mathematical equation (assuming Mathematical equation = 0) for Mathematical equation = 1 mrad (open circles) and 2 mrad (black bullets) and for (a) bw = 0.1%, (b) bw = 0.7% and (c) bw = 3%. Lines show the results of equation (13)[link] while points illustrate CAIN simulations (the error bars are too small to be visible).

4.2. Dependence on the electron beam energy spread

We now assume Mathematical equation = 0 mrad and we focus on the dependence of Mathematical equation on the energy spread of the electrons. We start again with the ratio Mathematical equation of the X-ray flux within a given energy bandwidth bw [see equation (8)[link]] and F0, the X-ray flux in the `ideal' case where Mathematical equation = Mathematical equation = 0 [see equation (3)[link]]. We assume that an angular selection α is applied. Only the first-order term in Mathematical equation will be kept (where Mathematical equation is defined in §3.2[link]). The quantities Mathematical equation and Mathematical equation are denoted by Mathematical equation and Mathematical equation, respectively. Then, depending on the relative values of Mathematical equation and bw, three configurations have to be distinguished: (i) bw < Mathematical equation < 2bw, (ii) 2bw < Mathematical equation and (iii) Mathematical equation < bw. Case (i) is illustrated in Fig. 11[link]. In this figure, the energy bandwidth is assumed to be centered at Mathematical equation = 1. The left panels correspond to Mathematical equation negative, the right ones to Mathematical equation positive. Hatched areas represent X-rays whose energy is within the selected energy bandwidth but which are rejected by the angular cut. As shown in this figure, the size of the overlap between the energy acceptance domain and the angular acceptance one depends on bw, α and Mathematical equation in the following way:

[Figure 11]
Figure 11
X-ray energy spectrum. The fraction of this spectrum which falls within the energy acceptance band is shown in green. The hatched bands represent X-rays which are eliminated because of the angular cutoff. Left panels correspond to Mathematical equation negative, right ones to Mathematical equation positive. (a) and (b) illustrate the cases where 0 < Mathematical equation < Mathematical equation, (c) and (d) where Mathematical equation < Mathematical equation < bw, and (e) and (f) where bw < Mathematical equation < bw + Mathematical equation.

(i) For increasing values of Mathematical equation, as long as Mathematical equation + bw < Mathematical equation, all X-rays accepted in the Mathematical equation energy band are emitted within the angular acceptance α as shown in panels (a) and (b).

(ii) For Mathematical equation − bw < Mathematical equation < bw, the fraction of X-rays remaining in the Mathematical equation angular acceptance band is (bw − Mathematical equation + Mathematical equation [see panels (c) and (d)].

(iii) The same fraction of X-rays pass the angular cut when bw < Mathematical equation < bw + Mathematical equation [panels (e) and (f)].

Similarly, the fraction of X-rays remaining in the Mathematical equation band in the configuration (ii) defined above is 1 and Mathematical equation for Mathematical equation < Mathematical equation − bw and Mathematical equation − bw < Mathematical equation < bw + Mathematical equation, respectively. In the (iii) configuration, this fraction is Mathematical equation for Mathematical equation < bw − Mathematical equation and (bw − Mathematical equation + Mathematical equation for bw − Mathematical equation < Mathematical equation < bw + Mathematical equation.

From this and from equation (5a)[link] which implies the following probability distribution,

Mathematical equation

the following expression of Mathematical equation as a function of Mathematical equation can be derived:

Mathematical equation

where Mathematical equation is given by equation (8)[link]. In the calculation of equation (14)[link], a simplification occurs which makes the dependence on minMathematical equation disappear, resulting in

Mathematical equation

CAIN simulations and results from equation (15)[link] are displayed in Fig. 12[link] where Mathematical equation is plotted as a function of Mathematical equation for several values of the angular and the energy acceptances.

[Figure 12]
Figure 12
The ratio Mathematical equation = Mathematical equation versus Mathematical equation, for Mathematical equation = 1 mrad (open circles) and 2 mrad (black bullets), and for (a) bw = 0.1%, (b) bw = 0.7% and (c) bw = 3%. Mathematical equation = 0 is assumed here. Lines are obtained by using the analytic expression (15)[link] while points are CAIN simulations (the error bars are too small to be visible).

4.3. Combined effect of the energy spread and the angular divergence of the electron beam

When both Mathematical equation and Mathematical equation must be taken into account to calculate the ratio Mathematical equation, this analytic formulation encounters a severe limitation for the following reason. When the incoming photons are backscattered by electrons whose energies are distributed according to equation (5a)[link], one may try to compute the X-ray flux in a way similar to that carried out in §4.1[link]. The bw term which comes in the Mathematical equation definition would have to be replaced by bweffective = bw + Mathematical equation, where Mathematical equation is defined in §3.2[link]. This would lead to an equation similar to equation (12)[link] with the Mathematical equation parameter occurring in the integrants and in the integrals' limits. The integration over Mathematical equation could still be performed, but the next step, namely an integral over Mathematical equation that takes into account the Mathematical equation distribution [equation (5a)[link]], cannot be performed analytically. Nevertheless, very good approximations can be obtained by employing equations previously established in this paper.

Indeed, if the electron beam angular divergence plays a dominant role with respect to the energy spread in the calculation of the X-ray flux within some acceptance cuts, a good approximation of Mathematical equation is obtained by using equation (13)[link] and assuming Mathematical equation = Mathematical equation, where Mathematical equation is the quadratic sum of bw and the standard deviation of Mathematical equation: bweff = Mathematical equation. On the contrary, when the electron beam energy spread is dominant with respect to the angular divergence, equation (15)[link] must be used wherein the quantity Mathematical equation is replaced by the quadratic sum of Mathematical equation and Mathematical equation, resulting in the substitution Mathematical equation Mathematical equation Mathematical equation + Mathematical equation.

CAIN simulations and results of the modified equations (13)[link] or (15)[link] are shown in Fig. 13[link] for several values of α and bw. The discontinuities seen in the lines mark the use of equations (15)[link] or (13)[link] with the appropriate adaptation described above. When Mathematical equation + bw < Mathematical equation, equation (15)[link] is used wherein Mathematical equation is replaced by Mathematical equation + Mathematical equation. Otherwise, equation (13)[link] is used where bw is replaced by Mathematical equation.

[Figure 13]
Figure 13
The ratio Mathematical equation = Mathematical equation as a function of Mathematical equation, for an electron energy spread Mathematical equation of 0.5% (circles) and 1.5% (squares) and for a selection angle Mathematical equation of 1 mrad (open symbols) and 2 mrad (full symbols). (a) bw = 0.1%. (b) bw = 0.7%. (c) bw = 3%. Lines are the analytic calculations (see text), points are CAIN simulations (the error bars are too small to be visible).

5. Additional comments and conclusion

We have derived analytic expressions for the total, the spectral and the angular X-ray fluxes of a Compton source according to the Compton kinematics and to the characteristics of the incoming electron and laser beams. The two dominant parameters governing the quality of such a source are the electron beam energy spread and its divergence. We point out a limitation of the analytic calculation of the flux Mathematical equation in a given energy bandwidth and a specified solid angle when both the energy spread and the divergence of the electron beam must be taken into account in the calculation. Nevertheless, the expressions of Mathematical equation obtained when either the energy spread or the angular divergence of the electron beam is taken into account can still be used with an appropriate modification.

Analytic expressions (11)[link], (13)[link] and (15)[link] provide the photon yield Mathematical equation within a given angular acceptance [equation (11)[link]] and the photon yield Mathematical equation within both a given angular acceptance and a given energy bandwidth [equations (13)[link] or (15)[link]]. Table 2[link] summarizes the validity domains of these equations in terms of the selected Compton kinematic region and according to the energy spread and the angular divergence of the two incoming beams as long as they are within the parameters ranges of current electron and laser beams (see Table 1[link]).

Table 2
Validity of equations (11)[link], (13)[link] and (15)[link] in terms of the parameters

The typical maximum values for current electron and laser beams shown in Table 1[link] are recalled. Each value indicates the upper limit of the parameter for which the equation is valid.

Parameters Mathematical equation (rad) bw Mathematical equation (rad) Mathematical equation (mrad) Mathematical equation Mathematical equation
e and typical laser values     0.25 10 A few % A few ‰
 
Equation (11)[link] 0.4   0.18 10 A few % A few ‰
Equations (13)[link] and (15)[link] Any 0.35 0.25 1 2–3%
†For the particular cases where Mathematical equation ≃ 1–10 mrad, Mathematical equation is valid but is overestimated by ∼0.5–5% via the term Mathematical equation (see §3.2[link]).

Within the large spectrum of X-ray applications in bio­medical, cultural heritage or material science, specific X-ray beams are required depending on the analysis technique and the sample to be used. For instance, a narrow energy bandwidth is required in most of the X-ray diffraction experiments (Dik et al., 2008[Dik, J., Janssens, K., Van Der Snickt, G., van der Loeff, L., Rickers, K. & Cotte, M. (2008). Anal. Chem. 80, 6436-6442.]) whereas therapy techniques such as stereotactic radiation therapy (Jacquet & Suortti, 2015[Jacquet, M. & Suortti, P. (2015). Phys. Med. 31, 596-600.]) can relax the constraint on the spectral width. Thus, for an incoming electron beam with a given emittance, it may be beneficial to minimize its transverse size even at the expense of its divergence. This could be the case for instance in experiments where a large X-ray number is the main requirement, or when an as small as possible source size is needed to carry out some analysis technique (such as phase-contrast imaging techniques). On the other hand, the electron beam divergence may be minimized at the expense of the transverse size when a quasi-monochromatic X-ray beam is required.

Analytic formulas (11)[link], (13)[link] and (15)[link] allow one to compute easily the spectral and spatial properties of an X-ray source based on photon backscattering, and highlight the beam parameters that play a key role for a given application. They should help when studying the feasibility of a particular experiment envisaged at some X-ray source.

Footnotes

1In the particular case of a Compton machine design such that Mathematical equation ≃ 1–10 mrad, the effect of the laser divergence leads to a reduction of Mathematical equation from a few per million to a few percent depending on Mathematical equation, Mathematical equation and bw. The largest effect occurs for Mathematical equation = 90° and Mathematical equation ≃ 10 mrad and would result for instance in a decrease of R0.1% and R3% by about 5% and 1%, respectively.

2We do not give here the expression of this third-order analytic formula since it is relatively heavy and since equation (11)[link] reproduces sufficiently well the simulations in our parameter range.

Acknowledgements

The authors are warmly grateful to Professor Jacques Haissinski for the many discussions and for his careful reading of the paper.

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